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PROSPECTS PROTONIC CERAMIC CELLS 2013
International Workshop
Protonic Ceramic Fuel Cells Status & Prospects
10– 12 July 2013
Hotel Mercure Centre
Montpellier, France
SCIENTIFIC PROGRAMME
Chair
Dr MARRONY Mathieu
European Institute for Energy Research - EIFER
Emmy-Noether Strasse 11
D-76131 Karlsruhe, Germany
ORAL SESSION
WEDNESDAY 10 JULY
8:30 – 9:00 Registration
9:00 – 9:15
M. Marrony - EIFER, Germany
Welcome
SPECIAL SESSION – FUNDAMENTAL STUDIES OF PCC HURDLES
CHAIRMAN: DR. M. MARRONY
9:15 – 10:00
10:00 – 10:45
Pr. R. Kee - Colorado School Mines, USA – Keynote Lecture
Transport theory in (mixed) protonic conductors
Dr. Y. Yamazaki - CIT, USA: Keynote Lecture
Proton trapping: a guide for proton conducting oxide electrolyte development
10:45 – 11:00 Coffee Break
11:00 – 11:45
11:45 – 12:30
Pr. P. Slater - Uni. Birmingham, United Kingdom – Keynote Lecture
Fundamental Studies of Fuel Cell Electrolyte Materials: Compositional Gradients and Effect of
Sintering Aids
Dr. P. Baranek - EDF R&D, France – Keynote Lecture
Illustrations of the atomic modeling used to understand the chemical stability and the protonic
diffusion in the PCFC electrolytes
12:30 – 14:00 Lunch
SESSION 1 - PROTON CONDUCTING OXIDE- BASED MATERIALS DEVELOPMENT: TOWARDS THE BEST PERFORMANCES...
CHAIRMAN: DR. G. COORS
BULK PROTON TRANSPORT MECHANISM AND ADVANCED PROCESSING STRATEGIES
14:00 - 14:45
14:45 - 15:15
15:15 – 15.45
15:45 – 16:15
Dr. R. Peng - USTC, China – Keynote Lecture
Ab-initio investigation of bulk transport and surface catalytic mechanisms on Ba 1-x ZrxO 3 cathode
materials in Solid Oxide Fuel Cells
Mr. F. Lenrick - Uni. Lund, Sweden
Transmission Electron Microscopy characterisation of thin film materials for protonic ceramic
fuel cells prepared by Focused Ion Beam
Pr. P. Colomban - ADIR UMPC, France
Autoclave testing of the chemical stability of ceramic membranes: surface reactions or bulk
protonation in perovskite frameworks?
Dr. Domingo Pérez-Coll - CSIC, Spain
Transport-Number Determination of a Protonic Ceramic Electrolyser Membrane via the Gorelov
Electrode Polarisation Correction
16:15 – 16:30 Coffee Break
GRAIN BOUNDARY RESISTANCE STUDIES, ELECTROLYTE DOPING STRATEGIES AND NOVEL STRUCTURE
CHAIRMAN: DR. G. TAILLADES
16:30 – 17:00
17:00 – 17:30
17:30 – 18:00
18:00 – 18:30
Dr. Y-C. Kim - KUTE, Korea
Proton migration at ∑3 1lt grain boundaries of barium zirconate and barium cerate
Dr. S. Ricote - Colorado School of Mines, USA
Grain boundary composition by atom probe tomography and conductivity of BaZr0.9Y0.1O3-δ
prepared by three different methods
Dr. Y. Liu - Uni. Nanjing, China
Improving proton conductivity of BaCe 0.9 Y 0.1 O 3-δ perovskite oxide protonic conductor through a
Pd catalytic approach
Pr. H. Matsumoto - Uni. Kyushu, Japan
Impact of transition metal doping on proton conduction properties of alkali earth cerates and
zirconates performance of infiltrated cathodes on protonic ceramic fuel cells
18:30 – 20:00 Poster session and appetizer
THURSDAY 11 JULY
GRAIN BOUNDARY RESISTANCE STUDIES, ELECTROLYTE DOPING STRATEGIES AND NOVEL STRUCTURE
CHAIRMAN: PR. J. ROZIÈRE
9:00 – 9:30
9:30- 10:00
10:00 – 10:30
Dr. S. Escolastico - CSIC-ITQ, Spain
Optimization of the hydrogen transport through La 5.5 WO 11.25−δ based membrane by selective
doping
Mr. F. Kinyanjui - DCBE, Uni. Chalmers, Sweden
Protonic conduction in oxygen deficient Ba 3 In 1.4 Y 0.3 M 0.3 ZrO 8 (M = Gd 3+ / Ga 3+ ) electrolytes
Dr. A. Smith - Uni. Birmingham, United Kingdom
Synthesis and Characterization of Oxyanion (Phosphate and Sulfate) doped Ba 2 Sc 2-y GayO 5 and
Sr 2 Sc 2-y GayO 5
10:30 – 10:45 Coffee Break
SESSION 2- PROTON CONDUCTING OXIDE - BASED CELL MANUFACTURING: TOWARDS THE BEST ARCHITECTURE...
CHAIRMAN: DR. N. BONANOS
NOVEL ANODE ARCHITECTURE
10:45 – 11:30
11:30 – 12:00
12:00 – 12:30
Dr. B-K. Kim - KIST, Korea: Invited speaker – Keynote Lecture
Novel Strategies to Fabricate an Anode Supported-Type Protonic Ceramic Fuel Cells (PCFCs) with
Dual Layer Electrolyte
Dr. M. Parco - TECNALIA, Spain
Development of anodes for proton conducting fuel cells by thermal spraying
Dr. D. Fagg - Uni. Aveiro, Portugal
Novel nitrate-free combustion route and electrochemical study of Ni-BaZr 0.85 Y 0.15 O 3-� anodes
12:30 – 14:00 Lunch
NOVEL CATHODE ARCHITECTURE AND CELL FABRICATION
CHAIRMAN: DR. S. RICOTE
14:00 – 14:30
14:30 – 15:00
15:00 – 15:30
15:30 – 16:00
Dr. S. Babiniec - Colorado School of Mines, USA
Performance of infiltrated cathodes on protonic ceramic fuel cells utilizing thin
BaCe 0.2 Zr 0.7 Y0.1O 3-δ electrolytes
Dr. L. Navarette - CSIC-ITQ, Spain
Tailor-made electrodes for LWO based PC-SOFC
Dr. P. Batocchi - ICMCB, France
Influence of water partial pressure on electrical and electrochemical properties of perovskite and
A2MO4-type oxides used as cathode materials for Protonic Ceramic Fuel Cell
Dr. E. Quarez - IMN, France
Compatibility of new proton conductor electrolytes with standard cathode materials
16:00 – 16:15 Coffee Break
SESSION 3 - SYSTEM ARCHITECTURE AND SCALING-UP
CHAIRMAN: DR. M. PARCO
16:15 – 17:00
17:00 – 17:30
17:30 – 18:00
18:00 – 18:30
Dr. ML. Fontaine - SINTEF, Norway – Keynote Lecture
Proton conducting fuel cells: interplay of Design, manufacturing and application
Dr. S. Molin - DTU, Denmark
High temperature corrosion of stainless steels for potential use as interconnects in Proton
Conducting Fuel Cell stacks
Dr. J. Dailly - EIFER, Germany
Recent results in up scaling approach strategy by wet chemical routes in EIFER
Mr. A. Manerbino - CoorsTek, USA
H 2 flux through dense tubular BaCe 0.2 Zr 0.7 Y 0.1 O 3-δ membranes as a function of temperature and
hydrogen partial pressure
20:00 Gala Dinner
FRIDAY 12 JULY
SESSION 4 - PROTON CONDUCTING OXIDE- BASED SYSTEM APPLICATIONS AND RELIABILITY: WHERE WE ARE?
CHAIRMAN: PR. H. MATSUMOTO
08:45 - 9:30
Pr M. Stoukides - CERTH, Greece – Keynote lecture
Applications of Proton Conductors in Heterogeneous Catalysis. The Example of Solid State
Ammonia Synthesis
HYDROGEN PUMPING APPLICATION /AMMONIA SYNTHESIS
9:30 – 10:00
10:00 - 10:30
10:30 – 11:00
Dr. A.Brandao - Uni. Aveiro, Portugal
Study of (SrLa)(NbV)O4-based composite as a hydrogen permeation membrane
Mr. S. Robinson - Colorado School of Mines, USA
Galvanic Hydrogen Flux and Fuel Cell Performance of Tubular Protonic Ceramic BaCe 0.2 Zr 0.7 Y 0.1 O 3-δ
Membranes
Dr G. Coors - CoorsTek, USA
One Million Liter per Day Gas-to-Liquid Refinery
11:00 – 11:15 Coffee Break
FUEL CELL APPLICATION
11:15 – 11:45
11:45 – 12:15
12:15 – 12:45
Dr. Y. Liu - Uni. Nanjing, China
A novel approach for substantially improving the sinterability of BaZr 0.4 Ce 0.4 Y 0.2 O 3-δ electrolyte for
fuel cells by impregnating green membrane with zinc nitrate as sintering aid
Dr. A. Magraso - Uni. Oslo, Norway
Performance of LaNbO 4 –based proton conducting fuel cell
Dr. H. Lee - Uni. Hanyang Korea
Enhanced electrochemical performance of BaZr 0.15 Ce 0.7 Y 0.15 O 3−δ -based proton-conducting solid
oxide fuel cells with continuous graded SSC-BZCY composite cathode by electrostatic spray slurry
deposition
HYDROGEN PRODUCTION APPLICATION
12:45 – 13:15
Dr. Y. Yoo - EME NRC, CA
PCC electrical performances & reliability under reversible profile: status and prospects
13:15 – 13:45 Conclusion
13:45 - 14:45 Lunch
POSTER SESSION
POSTER LIST
P1
P2
P3
P4
P5
P6
P7
P8
P9
Dr. S. Ricote - Colorado School of Mines, USA
Lan+1NinO3n+1 (n=1, 2, 3) as potential cathode materials for protonic ceramic fuel cells: hydration
properties and performance
Dr. P. Pasierb - AGH Uni. Krakow, Poland
Novel approach towards stable BaCeO 3 composite protonic conductors with high ionic conductivity
Dr. A. Lacz - AGH Uni. Krakow, Poland
Grain boundary modification of BaCeO 3 -based composites controlled by synthesis path
Dr. A. Chinelatto - CSIC, Spain
Synthesis, Structures and Proton Conductivity of the 12R-type Hexagonal Perovskite Solid Solution
Sr 3 NdNb 3-x TixO 12-δ (0 ≤ x ≤ 0.06)
Dr. N. Bonanos - DTU, Denmark
Impedance response of BaCe 0.2 Zr 0.7 Y 0.1 O 3-δ /Sr 0.95 Ti 0.9 Nb 0.1 O 3-δ (BCZY27/STN95) composite at nearambient
temperatures
Dr. C. Knee - Uni. Chalmers, Sweden
Role of B-site ion on Proton Conduction in Acceptor-doped Sm 2 B 2 O 7-δ (B = Ti, Sn, Zr and Ce)
Pyrochlores and C-type Compounds
Dr. M. Arab pour Yazdi - IRTES-LERMPS-UTBM, France
BaZr 1-x Y x O 3-α thin film deposited at high temperatures on commercial PCFC-anodes by reactive
magnetron sputtering
Dr. I. Antunes - CICECO, Uni. Aveiro, Portugal
Structure Property Relations of A- and B- site Pr doped BaTiO 3
Dr. C. Mortalo - CNR-IENI, Italy
Electrochemical investigation and chemical compatibility between Ln 2 NiO 4+� cathode materials and
BaCe 0.65 Zr 0.20 Y 0.15 O 3-δ electrolyte for PCFC application